Sird awakened the Unown at the Tanoby Ruins by solving the mystery shrouding it, a mystery that no-one could solve before. She used them to knocked out Lorelei's Slowking and her Jynx and surrounded Lorelei as a distraction, so her Starmie could camouflage itself into the rocks around them to prepare an attack.
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None of Unown's moves are known.